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The telecoms tycoon, dubbed the world's second-richest man by Forbes Magazine, is the second major investor this year to buy into the struggling media group.
Shares in the New York Times Company have fallen 33% over the last year.
Mr Slim's acquisition of 9.1 million shares means he and his family are the firm's third-largest investors.
Other key shareholders are the Sulzberger family - who own a controlling stake - and two hedge funds which bought stakes earlier this year.
Mr. Slim and the hedge funds, Harbinger Capital and Firebrand Partners, collectively hold more than 30% of firm's Class A shares. The Sulzberger family own 19%.
But the Sulzbergers, led by company chairman Arthur Sulzberger, control the publisher because they own nearly all of the firm's Class B shares, giving them the power to appoint most of the board.
(BBC)
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